Please use this identifier to cite or link to this item: http://hdl.handle.net/1942/18221
Title: Direct arylation as a versatile tool towards thiazolo- [5,4-d]thiazole-based semiconducting materials
Authors: KUDRJASOVA, Julija 
HERCKENS, Roald 
PENXTEN, Huguette 
ADRIAENSENS, Peter 
LUTSEN, Laurence 
VANDERZANDE, Dirk 
MAES, Wouter 
Issue Date: 2014
Source: ORGANIC & BIOMOLECULAR CHEMISTRY, 12 (26), p. 4663-4672
Abstract: A series of thiazolo[5,4-d]thiazole-based small molecule organic optoelectronic materials is synthesized via a straightforward microwave-activated Pd-catalyzed C–H arylation protocol. The procedure allows us to obtain extended 2,5-dithienylthiazolo[5,4-d]thiazole chromophores with tailor-made energy levels and absorption patterns, depending on the introduced (het)aryl moieties and the molecular (a)symmetry, by shortened sequences without organometallic intermediates. The synthesized materials can be applied as either electron donor or electron acceptor light-harvesting materials in molecular bulk heterojunction organic solar cells.
Document URI: http://hdl.handle.net/1942/18221
ISSN: 1477-0520
e-ISSN: 1477-0539
DOI: 10.1039/c4ob00360h
ISI #: 000337139800019
Rights: This journal is © The Royal Society of Chemistry 2014.
Category: A1
Type: Journal Contribution
Validations: ecoom 2015
Appears in Collections:Research publications

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