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http://hdl.handle.net/1942/18221
Title: | Direct arylation as a versatile tool towards thiazolo- [5,4-d]thiazole-based semiconducting materials | Authors: | KUDRJASOVA, Julija HERCKENS, Roald PENXTEN, Huguette ADRIAENSENS, Peter LUTSEN, Laurence VANDERZANDE, Dirk MAES, Wouter |
Issue Date: | 2014 | Source: | ORGANIC & BIOMOLECULAR CHEMISTRY, 12 (26), p. 4663-4672 | Abstract: | A series of thiazolo[5,4-d]thiazole-based small molecule organic optoelectronic materials is synthesized via a straightforward microwave-activated Pd-catalyzed C–H arylation protocol. The procedure allows us to obtain extended 2,5-dithienylthiazolo[5,4-d]thiazole chromophores with tailor-made energy levels and absorption patterns, depending on the introduced (het)aryl moieties and the molecular (a)symmetry, by shortened sequences without organometallic intermediates. The synthesized materials can be applied as either electron donor or electron acceptor light-harvesting materials in molecular bulk heterojunction organic solar cells. | Document URI: | http://hdl.handle.net/1942/18221 | ISSN: | 1477-0520 | e-ISSN: | 1477-0539 | DOI: | 10.1039/c4ob00360h | ISI #: | 000337139800019 | Rights: | This journal is © The Royal Society of Chemistry 2014. | Category: | A1 | Type: | Journal Contribution | Validations: | ecoom 2015 |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
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Kudrjasova, OBC 2014, 4663.pdf Restricted Access | 1.08 MB | Adobe PDF | View/Open Request a copy |
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