Please use this identifier to cite or link to this item:
http://hdl.handle.net/1942/21799
Full metadata record
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Tait, J. G. | - |
dc.contributor.author | Manghooli, S. | - |
dc.contributor.author | Qiu, W. | - |
dc.contributor.author | Rakocevic, L. | - |
dc.contributor.author | Kootstra, L. | - |
dc.contributor.author | Jaysankar, M. | - |
dc.contributor.author | de la Huerta, C. A. Masse | - |
dc.contributor.author | Paetzold, U. W. | - |
dc.contributor.author | Gehlhaar, R. | - |
dc.contributor.author | Cheyns, D. | - |
dc.contributor.author | Heremans, P. | - |
dc.contributor.author | POORTMANS, Jef | - |
dc.date.accessioned | 2016-07-18T09:33:16Z | - |
dc.date.available | 2016-07-18T09:33:16Z | - |
dc.date.issued | 2016 | - |
dc.identifier.citation | JOURNAL OF MATERIALS CHEMISTRY A, 4 (10), p. 3792-3797 | - |
dc.identifier.issn | 2050-7488 | - |
dc.identifier.uri | http://hdl.handle.net/1942/21799 | - |
dc.description.abstract | Transitioning perovskite photovoltaics from the rapid progress in lab-scale devices to industrially viable large area modules is a key challenge for the economic breakthrough of the technology. In this work, we demonstrate ultrasonic spray coating as a scalable and versatile linear deposition technique for high efficiency perovskite photovoltaics. We show the versatility of concurrently pumped ultrasonic spray coating by rapidly and precisely optimizing precursor ratios based on PbCl2, Pb(CH3CO2)(2)center dot 3H(2)O, PbBr2, CH3NH3Br, and CH3NH3I to achieve highly crystalline and pinhole-free layers. Initial power conversion efficiencies of 15.7% for small scale devices and 11.7% for 3.8 cm(2) modules were achieved with current-voltage sweeps and tracked to 13.4% for devices and 10.4% for modules under continuous illumination and bias at the maximum power point. Process versatility is further demonstrated with the in situ bandgap control in CH3NH3PbIXBr3-X layers. | - |
dc.description.sponsorship | This work was supported in part by the Flemish Government: Department of Economics, Science and Innovation. The work of J. G. Tait was supported by the Natural Sciences Engineering and Research Council of Canada under CGSD3-454097-2014. The work of U. W. Paetzold was supported by the German Academic Exchange Service. The authors declare no competing financial interests. | - |
dc.language.iso | en | - |
dc.publisher | ROYAL SOC CHEMISTRY | - |
dc.rights | This journal is © The Royal Society of Chemistry 2016 | - |
dc.title | Rapid composition screening for perovskite photovoltaics via concurrently pumped ultrasonic spray coating | - |
dc.type | Journal Contribution | - |
dc.identifier.epage | 3797 | - |
dc.identifier.issue | 10 | - |
dc.identifier.spage | 3792 | - |
dc.identifier.volume | 4 | - |
local.format.pages | 6 | - |
local.bibliographicCitation.jcat | A1 | - |
dc.description.notes | [Tait, J. G.; Manghooli, S.; Qiu, W.; Rakocevic, L.; Kootstra, L.; Jaysankar, M.; de la Huerta, C. A. Masse; Paetzold, U. W.; Gehlhaar, R.; Cheyns, D.; Heremans, P.; Poortmans, J.] IMEC, Kapeldreef 75, B-3001 Leuven, Belgium. [Tait, J. G.; Qiu, W.; Rakocevic, L.; Jaysankar, M.; Heremans, P.; Poortmans, J.] KULeuven, Dept Elect Eng, Leuven, Belgium. [Manghooli, S.] Politecn Milan, Dept Elect Eng, Milan, Italy. [Kootstra, L.] Delft Univ Technol, Dept Appl Sci, Delft, Netherlands. [de la Huerta, C. A. Masse] Inst Natl Sci Appl Lyon, Lyon, France. [Poortmans, J.] Univ Hasselt, Dept Mat, Hasselt, Belgium. | - |
local.publisher.place | CAMBRIDGE | - |
local.type.refereed | Refereed | - |
local.type.specified | Article | - |
dc.identifier.doi | 10.1039/c6ta00739b | - |
dc.identifier.isi | 000371967000024 | - |
item.validation | ecoom 2017 | - |
item.accessRights | Restricted Access | - |
item.fullcitation | Tait, J. G.; Manghooli, S.; Qiu, W.; Rakocevic, L.; Kootstra, L.; Jaysankar, M.; de la Huerta, C. A. Masse; Paetzold, U. W.; Gehlhaar, R.; Cheyns, D.; Heremans, P. & POORTMANS, Jef (2016) Rapid composition screening for perovskite photovoltaics via concurrently pumped ultrasonic spray coating. In: JOURNAL OF MATERIALS CHEMISTRY A, 4 (10), p. 3792-3797. | - |
item.fulltext | With Fulltext | - |
item.contributor | Tait, J. G. | - |
item.contributor | Manghooli, S. | - |
item.contributor | Qiu, W. | - |
item.contributor | Rakocevic, L. | - |
item.contributor | Kootstra, L. | - |
item.contributor | Jaysankar, M. | - |
item.contributor | de la Huerta, C. A. Masse | - |
item.contributor | Paetzold, U. W. | - |
item.contributor | Gehlhaar, R. | - |
item.contributor | Cheyns, D. | - |
item.contributor | Heremans, P. | - |
item.contributor | POORTMANS, Jef | - |
crisitem.journal.issn | 2050-7488 | - |
crisitem.journal.eissn | 2050-7496 | - |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
---|---|---|---|---|
c6ta00739b.pdf Restricted Access | Published version | 1.47 MB | Adobe PDF | View/Open Request a copy |
SCOPUSTM
Citations
68
checked on Sep 2, 2020
WEB OF SCIENCETM
Citations
119
checked on May 8, 2024
Page view(s)
58
checked on Sep 7, 2022
Download(s)
52
checked on Sep 7, 2022
Google ScholarTM
Check
Altmetric
Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.