Please use this identifier to cite or link to this item:
http://hdl.handle.net/1942/30137
Title: | In Situ Mechanical Analysis of the Nanoscopic Solid Electrolyte Interphase on Anodes of Li-Ion Batteries | Authors: | MOEREMANS, Boaz Cheng, Hsiu-Wei Merola, Claudia Hu, Qingyun Oezaslan, Mehtap SAFARI, Momo VAN BAEL, Marlies HARDY, An Valtiner, Markus RENNER, Frank |
Issue Date: | 2019 | Publisher: | WILEY | Source: | ADVANCED SCIENCE, 6(16) | Abstract: | The interfacial decomposition products forming the so-called solid-electrolyte interphase (SEI) significantly determine the destiny of a Li-ion battery. Ultimate knowledge of its detailed behavior and better control are required for higher rates, longer life-time, and increased safety. Employing an electrochemical surface force apparatus, it is possible to control the growth and to investigate the mechanical properties of an SEI in a lithium-ion battery environment. This new approach is here introduced on a gold model system and reveals a compressible film at all stages of SEI growth. The demonstrated methodology provides a unique tool for analyzing electrochemical battery interfaces, in particular in view of alternative electrolyte formulations and artificial interfaces. | Notes: | [Moeremans, Boaz; Safari, Mohammadhosein; Van Bael, Marlies K.; Hardy, An; Renner, Frank Uwe] Hasselt Univ, Inst Mat Res, BE-3590 Diepenbeek, Belgium. [Moeremans, Boaz; Cheng, Hsiu-Wei; Merola, Claudia; Hu, Qingyun; Valtiner, Markus] Max Planck Inst Eisenforsch GmbH, D-40237 Dusseldorf, Germany. [Moeremans, Boaz; Valtiner, Markus] TU Bergakad Freiberg, Inst Phys Chem 2, D-09599 Freiberg, Germany. [Cheng, Hsiu-Wei; Merola, Claudia; Hu, Qingyun; Valtiner, Markus] Vienna Univ Technol, Appl Interface Phys, Inst Appl Phys, A-1040 Vienna, Austria. [Oezaslan, Mehtap] Carl von Ossietzky Univ Oldenburg, Phys Chem, Electrocatalysis, D-26111 Oldenburg, Germany. [Safari, Mohammadhosein; Van Bael, Marlies K.; Hardy, An; Renner, Frank Uwe] IMEC, Div IMOMEC, BE-3590 Diepenbeek, Belgium. | Keywords: | Li-ion batteries;polymers;soft matter;solid–electrolyte interphases;surface force apparatus | Document URI: | http://hdl.handle.net/1942/30137 | e-ISSN: | 2198-3844 | DOI: | 10.1002/advs.201900190 | ISI #: | 000482048100003 | Rights: | 2019 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited. | Category: | A1 | Type: | Journal Contribution | Validations: | ecoom 2020 |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
---|---|---|---|---|
Moeremans_et_al-2019-Advanced_Science.pdf | Published version | 2.56 MB | Adobe PDF | View/Open |
SCOPUSTM
Citations
5
checked on Sep 2, 2020
WEB OF SCIENCETM
Citations
25
checked on Oct 13, 2024
Page view(s)
72
checked on Sep 7, 2022
Download(s)
16
checked on Sep 7, 2022
Google ScholarTM
Check
Altmetric
Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.