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http://hdl.handle.net/1942/34608
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DC Field | Value | Language |
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dc.contributor.author | KAYAHAN, Emine | - |
dc.contributor.author | JACOBS, Mathias | - |
dc.contributor.author | BRAEKEN, Leen | - |
dc.contributor.author | THOMASSEN, Leen | - |
dc.contributor.author | Kuhn, Simon | - |
dc.contributor.author | van Gerven, Tom | - |
dc.contributor.author | LEBLEBICI, Mumin enis | - |
dc.date.accessioned | 2021-08-05T11:37:20Z | - |
dc.date.available | 2021-08-05T11:37:20Z | - |
dc.date.issued | 2020 | - |
dc.date.submitted | 2021-07-08T10:12:01Z | - |
dc.identifier.citation | Beilstein journal of organic chemistry, 16 , p. 2484 -2504 | - |
dc.identifier.uri | http://hdl.handle.net/1942/34608 | - |
dc.description.abstract | Photochemical activation routes are gaining the attention of the scientific community since they can offer an alternative to the tradi-tional chemical industry that mainly utilizes thermochemical activation of molecules. Photoreactions are fast and selective, which would potentially reduce the downstream costs significantly if the process is optimized properly. With the transition towards green chemistry, the traditional batch photoreactor operation is becoming abundant in this field. Process intensification efforts led to microand mesostructured flow photoreactors. In this work, we are reviewing structured photoreactors by elaborating on the bottleneck of this field: the development of an efficient scale-up strategy. In line with this, microand mesostructured bench-scale photoreactors were evaluated based on a new benchmark called photochemical space time yield (mol.day(-1).kW(-1)), which takes into account the energy efficiency of the photoreactors. It was manifested that along with the selection of the photoreactor dimensions and an appropriate light source, optimization of the process conditions, such as the residence time and the concentration of the photoactive molecule is also crucial for an efficient photoreactor operation. In this paper, we are aiming to give a comprehensive understanding for scale-up strategies by benchmarking selected photoreactors and by discussing transport phenomena in several other photoreactors. | - |
dc.language.iso | en | - |
dc.publisher | - | |
dc.subject.other | microreactor | - |
dc.subject.other | microreactor scale-up | - |
dc.subject.other | monolith reactors | - |
dc.subject.other | packed bed reactor | - |
dc.subject.other | photoreactor scale-up | - |
dc.title | Dawn of a new era in industrial photochemistry: the scale-up of micro- and mesostructured photoreactors | - |
dc.type | Journal Contribution | - |
dc.identifier.epage | 2504 | - |
dc.identifier.spage | 2484 | - |
dc.identifier.volume | 16 | - |
local.bibliographicCitation.jcat | A1 | - |
local.type.refereed | Refereed | - |
local.type.specified | Review | - |
dc.identifier.doi | 10.3762/bjoc.16.202 | - |
dc.identifier.isi | WOS:000577170000001 | - |
dc.contributor.orcid | Kuhn, Simon/0000-0002-2816-0060; Kayahan, Emine/0000-0002-5286-624X; | - |
dc.contributor.orcid | Thomassen, Leen C. J./0000-0002-4970-7475; Leblebici, Mumin | - |
dc.contributor.orcid | Enis/0000-0003-4599-9412; Jacobs, Mathias/0000-0002-9865-746X | - |
local.provider.type | wosris | - |
local.uhasselt.international | no | - |
item.fullcitation | KAYAHAN, Emine; JACOBS, Mathias; BRAEKEN, Leen; THOMASSEN, Leen; Kuhn, Simon; van Gerven, Tom & LEBLEBICI, Mumin enis (2020) Dawn of a new era in industrial photochemistry: the scale-up of micro- and mesostructured photoreactors. In: Beilstein journal of organic chemistry, 16 , p. 2484 -2504. | - |
item.contributor | KAYAHAN, Emine | - |
item.contributor | JACOBS, Mathias | - |
item.contributor | BRAEKEN, Leen | - |
item.contributor | THOMASSEN, Leen | - |
item.contributor | Kuhn, Simon | - |
item.contributor | van Gerven, Tom | - |
item.contributor | LEBLEBICI, Mumin enis | - |
item.accessRights | Open Access | - |
item.fulltext | With Fulltext | - |
crisitem.journal.issn | 1860-5397 | - |
crisitem.journal.eissn | 1860-5397 | - |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
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1860-5397-16-202.pdf | Published version | 7.88 MB | Adobe PDF | View/Open |
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