Please use this identifier to cite or link to this item: http://hdl.handle.net/1942/35757
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dc.contributor.authorHoang, Nong, V-
dc.contributor.authorNikolis, Vasileios C.-
dc.contributor.authorBaisinger, Lukasz-
dc.contributor.authorVANDEWAL, Koen-
dc.contributor.authorPshenichnikov, Maxim S.-
dc.date.accessioned2021-11-04T09:06:12Z-
dc.date.available2021-11-04T09:06:12Z-
dc.date.issued2021-
dc.date.submitted2021-10-28T14:06:29Z-
dc.identifier.citationPCCP. Physical chemistry chemical physics (Print), 23 (37) , p. 20848 -20853-
dc.identifier.issn1463-9076-
dc.identifier.urihttp://hdl.handle.net/1942/35757-
dc.description.abstractSingle-material organic solar cells have recently attracted research attention due to their simplicity, morphological robustness and high yield of exciton dissociation. Using alpha-sexithiophene as a model system, we show that the single-event probability of the exciton dissociation at the boundaries of polycrystalline domains with different molecular orientation is extremely low (similar to 0.5%), while a high efficiency of charge generation is gained via hundred-fold crossings of the domain boundaries due to the long exciton diffusion length (similar to 45 nm).-
dc.description.sponsorshipN. V. H. and M. S. P. thank F. de Haan for writing the code for kinetic Monte-Carlo simulations and general laboratory assistance. The SEPOMO network participants (especially D. Beljonne) are acknowledged for numerous discussions. We are indebted to A. A. Bakulin for constructive criticism upon reading the manuscript. N. V. H. thanks K. Leo for hospitality during his secondment stay at Dresden Integrated Center for Applied Physics and Photonic Materials. N. V. H., K. V. and M. S. P. acknowledge funding from the European Union’s Horizon 2020 research and innovation program under Marie Sklodowska Curie Grant Agreement No. 722651 (SEPOMO).-
dc.language.isoen-
dc.publisherROYAL SOC CHEMISTRY-
dc.rightsOpen Access Article. Published on 07 September 2021. Downloaded on 11/4/2021 9:03:51 AM. This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence-
dc.titleDiffusion-enhanced exciton dissociation in single-material organic solar cells-
dc.typeJournal Contribution-
dc.identifier.epage20853-
dc.identifier.issue37-
dc.identifier.spage20848-
dc.identifier.volume23-
local.format.pages6-
local.bibliographicCitation.jcatA1-
dc.description.notesPshenichnikov, MS (corresponding author), Univ Groningen, Zernike Inst Adv Mat, Nijenbargh 4, NL-9747 AG Groningen, Netherlands.-
dc.description.notesm.s.pchenitchnikov@rug.nl-
local.publisher.placeTHOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND-
local.type.refereedRefereed-
local.type.specifiedArticle-
local.type.programmeH2020-
local.relation.h2020722651-
dc.identifier.doi10.1039/d1cp03328j-
dc.identifier.pmid34546274-
dc.identifier.isiWOS:000697468300001-
dc.contributor.orcidVandewal, Koen/0000-0001-5471-383X-
dc.identifier.eissn1463-9084-
local.provider.typewosris-
local.uhasselt.uhpubyes-
local.description.affiliation[Hoang, Nong, V; Pshenichnikov, Maxim S.] Univ Groningen, Zernike Inst Adv Mat, Nijenbargh 4, NL-9747 AG Groningen, Netherlands.-
local.description.affiliation[Nikolis, Vasileios C.; Baisinger, Lukasz; Vandewal, Koen] Tech Univ Dresden, Dresden Integrated Ctr Appl Phys & Photon Mat, Nothnitzer Str 61, D-01187 Dresden, Germany.-
local.description.affiliation[Nikolis, Vasileios C.] Heliatek GmbH, Treidlerstr 3, D-01139 Dresden, Germany.-
local.description.affiliation[Vandewal, Koen] Hasselt Univ, Inst Mat Res IMO IMOMEC, Wetenschapspk 1, B-3590 Diepenbeek, Belgium.-
local.uhasselt.internationalyes-
item.fullcitationHoang, Nong, V; Nikolis, Vasileios C.; Baisinger, Lukasz; VANDEWAL, Koen & Pshenichnikov, Maxim S. (2021) Diffusion-enhanced exciton dissociation in single-material organic solar cells. In: PCCP. Physical chemistry chemical physics (Print), 23 (37) , p. 20848 -20853.-
item.fulltextWith Fulltext-
item.validationecoom 2022-
item.accessRightsOpen Access-
item.contributorHoang, Nong, V-
item.contributorNikolis, Vasileios C.-
item.contributorBaisinger, Lukasz-
item.contributorVANDEWAL, Koen-
item.contributorPshenichnikov, Maxim S.-
crisitem.journal.issn1463-9076-
crisitem.journal.eissn1463-9084-
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