Please use this identifier to cite or link to this item:
http://hdl.handle.net/1942/36018
Full metadata record
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Aydin, E | - |
dc.contributor.author | Liu, J | - |
dc.contributor.author | Ugur, E | - |
dc.contributor.author | Azmi, R | - |
dc.contributor.author | Harrison, GT | - |
dc.contributor.author | Hou, Y | - |
dc.contributor.author | Chen , B | - |
dc.contributor.author | Zhumagali, S | - |
dc.contributor.author | De Bastiani, M | - |
dc.contributor.author | Wang, MC | - |
dc.contributor.author | Raja, W | - |
dc.contributor.author | Allen, TG | - |
dc.contributor.author | Rehman, AU | - |
dc.contributor.author | Subbiah, AS | - |
dc.contributor.author | Babics, M | - |
dc.contributor.author | BABAYIGIT, Aslihan | - |
dc.contributor.author | Isikgor, FH | - |
dc.contributor.author | Wang, K | - |
dc.contributor.author | Van Kerschaver, E | - |
dc.contributor.author | Tsetseris, L | - |
dc.contributor.author | Sargent, EH | - |
dc.contributor.author | Laquai, F | - |
dc.contributor.author | De Wolf , S | - |
dc.date.accessioned | 2021-12-02T14:30:01Z | - |
dc.date.available | 2021-12-02T14:30:01Z | - |
dc.date.issued | 2021 | - |
dc.date.submitted | 2021-09-13T14:13:30Z | - |
dc.identifier.citation | Energy & environmental science (Print), 14 (8) , p. 4377 -4390 | - |
dc.identifier.issn | 1754-5692 | - |
dc.identifier.uri | http://hdl.handle.net/1942/36018 | - |
dc.description.abstract | Translating the high power conversion efficiencies of single-junction perovskite solar cells in their classic, non-inverted (n-i-p) architecture to efficient monolithic n-i-p perovskite/silicon tandem solar cells with high current densities has been a persistent challenge due to the lack of low-temperature processable, chemically-insoluble contact materials with appropriate polarity and sufficient optical transparency. To address this, we developed sputtered amorphous niobium oxide (a-NbOx) with ligand-bridged C-60 as an efficient electron-selective contact, deposited on the textured-silicon bottom cell. For the sunward, hole-selective contact we implemented a stack of molecularly doped broadband transparent evaporated 2,2 ',7,7 '-tetra(N,N-di-p-tolyl)amino-9,9-spirobifluorene (spiro-TTB) and atomic layer deposited vanadium oxide, which further enhances the device quantum efficiency. Combining these contact materials with two-dimensional perovskite passivation on the micrometer-thick solution-processed perovskite top cell yields 27% efficient monolithic n-i-p perovskite/silicon tandem solar cells, which represents one of the highest power conversion efficiencies reported on pyramidal textured crystalline silicon bottom cells, and the highest with this polarity. | - |
dc.description.sponsorship | The authors would like to thanks to Nini Wei for the TEM images; funding: the research reported in this publication was supported by funding from King Abdullah University of Science and Technology (KAUST) under award no. OSR-CARF/CCF-3079 and award no. IED OSR-2019-4208. | - |
dc.language.iso | en | - |
dc.publisher | ROYAL SOC CHEMISTRY | - |
dc.rights | The Royal Society of Chemistry 2021 Open access Article. | - |
dc.title | Ligand-bridged charge extraction and enhanced quantum efficiency enable efficient n-i-p perovskite/silicon tandem solar cells | - |
dc.type | Journal Contribution | - |
dc.identifier.epage | 4390 | - |
dc.identifier.issue | 8 | - |
dc.identifier.spage | 4377 | - |
dc.identifier.volume | 14 | - |
local.bibliographicCitation.jcat | A1 | - |
local.publisher.place | THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND | - |
local.type.refereed | Refereed | - |
local.type.specified | Article | - |
dc.identifier.doi | 10.1039/d1ee01206a | - |
dc.identifier.isi | 000670654700001 | - |
dc.identifier.eissn | 1754-5706 | - |
local.provider.type | Web of Science | - |
local.uhasselt.international | yes | - |
item.validation | ecoom 2022 | - |
item.contributor | Aydin, E | - |
item.contributor | Liu, J | - |
item.contributor | Ugur, E | - |
item.contributor | Azmi, R | - |
item.contributor | Harrison, GT | - |
item.contributor | Hou, Y | - |
item.contributor | Chen , B | - |
item.contributor | Zhumagali, S | - |
item.contributor | De Bastiani, M | - |
item.contributor | Wang, MC | - |
item.contributor | Raja, W | - |
item.contributor | Allen, TG | - |
item.contributor | Rehman, AU | - |
item.contributor | Subbiah, AS | - |
item.contributor | Babics, M | - |
item.contributor | BABAYIGIT, Aslihan | - |
item.contributor | Isikgor, FH | - |
item.contributor | Wang, K | - |
item.contributor | Van Kerschaver, E | - |
item.contributor | Tsetseris, L | - |
item.contributor | Sargent, EH | - |
item.contributor | Laquai, F | - |
item.contributor | De Wolf , S | - |
item.accessRights | Open Access | - |
item.fullcitation | Aydin, E; Liu, J; Ugur, E; Azmi, R; Harrison, GT; Hou, Y; Chen , B; Zhumagali, S; De Bastiani, M; Wang, MC; Raja, W; Allen, TG; Rehman, AU; Subbiah, AS; Babics, M; BABAYIGIT, Aslihan; Isikgor, FH; Wang, K; Van Kerschaver, E; Tsetseris, L; Sargent, EH; Laquai, F & De Wolf , S (2021) Ligand-bridged charge extraction and enhanced quantum efficiency enable efficient n-i-p perovskite/silicon tandem solar cells. In: Energy & environmental science (Print), 14 (8) , p. 4377 -4390. | - |
item.fulltext | With Fulltext | - |
crisitem.journal.issn | 1754-5692 | - |
crisitem.journal.eissn | 1754-5706 | - |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
---|---|---|---|---|
Ligand-bridged charge extraction and enhanced quantum efficiency enable efficient n–i–p perovskite_silicon tandem solar cells.pdf | Published version | 8.97 MB | Adobe PDF | View/Open |
WEB OF SCIENCETM
Citations
71
checked on Apr 30, 2024
Page view(s)
66
checked on Sep 7, 2022
Google ScholarTM
Check
Altmetric
Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.