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http://hdl.handle.net/1942/36504Full metadata record
| DC Field | Value | Language |
|---|---|---|
| dc.contributor.author | GUEIBE, Christophe | - |
| dc.contributor.author | Rutten, Jos | - |
| dc.contributor.author | CAMPS, Johan | - |
| dc.contributor.author | Moyaux, Dominique | - |
| dc.contributor.author | SCHROEYERS, Wouter | - |
| dc.contributor.author | Auer, Matthias | - |
| dc.contributor.author | SCHREURS, Sonja | - |
| dc.date.accessioned | 2022-01-17T12:20:01Z | - |
| dc.date.available | 2022-01-17T12:20:01Z | - |
| dc.date.issued | 2022 | - |
| dc.date.submitted | 2022-01-06T14:03:35Z | - |
| dc.date.submitted | 2022-01-06T14:03:35Z | - |
| dc.identifier.citation | Process safety and environmental protection, 158 , p. 576 -588 | - |
| dc.identifier.uri | http://hdl.handle.net/1942/36504 | - |
| dc.description.abstract | Atmospheric radioxenon releases from fission-based medical isotope production facilities are the main contributors to the radioxenon background being observed in the International Monitoring System (IMS) for the verification of the Comprehensive Nuclear-Test-Ban Treaty. This background is impacting the detection capability of the IMS network for potential nuclear explosions. Reducing the radioxenon emissions from these facilities requires the optimization of the corresponding filtration process. The investigation of more efficient Xe adsorption materials than Activated Carbon (AC), which is currently used for this application, can play an important role for such an optimization. In this work, the Xe adsorption capacity of silver-exchanged zeolites (AgZs) is compared to the one of ACs in relevant conditions for fission-based medical isotope production facilities. The most promising AgZ candidate, a silver-exchanged titanosilicate (Ag-ETS-10), is investigated in more detail for its application to further reduce radioxenon releases. As operational conditions depend on the production and off-gas treatment processes, the effect of Xe concentration, flow rate, temperature and moisture on the Xe adsorption in Ag-ETS-10 is reported. Furthermore, since AgZs are far more expensive than ACs, it is crucial to be able to regenerate the material, whilst maintaining its full Xe adsorption properties for successive reuse. Accordingly, the durability of Ag-ETS-10 is investigated with regard to desorption and adsorption cycles but also with regard to gamma irradiation. | - |
| dc.language.iso | en | - |
| dc.publisher | Elsevier | - |
| dc.rights | © 2021 Institution of Chemical Engineers. Published by Elsevier B.V. All rights reserved. | - |
| dc.subject.other | Xenon adsorption | - |
| dc.subject.other | Regeneration | - |
| dc.subject.other | Silver-exchanged zeolite | - |
| dc.subject.other | Activated carbon | - |
| dc.subject.other | CTBT verification | - |
| dc.subject.other | Medical isotope production facilities | - |
| dc.title | Application of silver-exchanged zeolite for radioxenon mitigation at fission-based medical isotope production facilities | - |
| dc.type | Journal Contribution | - |
| dc.identifier.epage | 588 | - |
| dc.identifier.spage | 576 | - |
| dc.identifier.volume | 158 | - |
| local.bibliographicCitation.jcat | A1 | - |
| local.publisher.place | RADARWEG 29, 1043 NX AMSTERDAM, NETHERLANDS | - |
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| local.type.refereed | Refereed | - |
| local.type.specified | Article | - |
| dc.identifier.doi | 10.1016/j.psep.2021.12.031 | - |
| dc.identifier.isi | WOS:000740947300002 | - |
| local.provider.type | - | |
| local.uhasselt.uhpub | yes | - |
| local.uhasselt.international | no | - |
| item.fullcitation | GUEIBE, Christophe; Rutten, Jos; CAMPS, Johan; Moyaux, Dominique; SCHROEYERS, Wouter; Auer, Matthias & SCHREURS, Sonja (2022) Application of silver-exchanged zeolite for radioxenon mitigation at fission-based medical isotope production facilities. In: Process safety and environmental protection, 158 , p. 576 -588. | - |
| item.validation | ecoom 2023 | - |
| item.fulltext | With Fulltext | - |
| item.accessRights | Open Access | - |
| item.contributor | GUEIBE, Christophe | - |
| item.contributor | Rutten, Jos | - |
| item.contributor | CAMPS, Johan | - |
| item.contributor | Moyaux, Dominique | - |
| item.contributor | SCHROEYERS, Wouter | - |
| item.contributor | Auer, Matthias | - |
| item.contributor | SCHREURS, Sonja | - |
| crisitem.journal.issn | 0957-5820 | - |
| crisitem.journal.eissn | 1744-3598 | - |
| Appears in Collections: | Research publications | |
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| 2022_Gueibe_Application of AgZ for radioxenon mitigation at fission based MIPFs.pdf Restricted Access | Published version | 6.5 MB | Adobe PDF | View/Open Request a copy |
| Manuscript_Application of AgZ for radioxenon mitigation_Revised_Clean.pdf | Peer-reviewed author version | 1.52 MB | Adobe PDF | View/Open |
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