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http://hdl.handle.net/1942/40036| Title: | Photocatalytic and Electrocatalytic Generation of Hydrogen Peroxide: Principles, Catalyst Design and Performance | Authors: | Guo, Yan Tong, Xili YANG, Nianjun |
Issue Date: | 2023 | Publisher: | SHANGHAI JIAO TONG UNIV PRESS | Source: | Nano-Micro Letters, 15 (1) (Art N° 77) | Abstract: | Hydrogen peroxide -(H2O2) is a high-demand organic chemical reagent and has been widely used in various modern industrial applications. Currently, the prominent method for the preparation of -H2O2 is the anthraquinone oxidation. Unfortunately, it is not conducive to economic and sustainable development since it is a complex process and involves unfriendly environment and potential hazards. In this context, numerous approaches have been developed to synthesize -H2O2. Among them, photo/electro-catalytic ones are considered as two of the most promising manners for on- site synthesis of -H2O2. These alternatives are sustainable in that only water or -O-2 is required. Namely, water oxidation (WOR) or oxygen reduction (ORR) reactions can be further coupled with clean and sustainable energy. For photo/electro-catalytic reactions for -H2O2 generation, the design of the catalysts is extremely important and has been extensively conducted with an aim to obtain ultimate catalytic performance. This article overviews the basic principles of WOR and ORR, followed by the summary of recent progresses and achievements on the design and performance of various photo/electro-catalysts for -H2O2 generation. The related mechanisms for these approaches are highlighted from theoretical and experimental aspects. Scientific challenges and opportunities of engineering photo/electro-catalysts for -H2O2 generation are also outlined and discussed. | Notes: | Tong, XL (corresponding author), Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Peoples R China.; Yang, NJ (corresponding author), Univ Siegen, Inst Mat Engn, D-57076 Siegen, Germany.; Yang, NJ (corresponding author), Hasselt Univ, Dept Chem, B-3590 Diepenbeek, Belgium.; Yang, NJ (corresponding author), Hasselt Univ, IMO IMOMEC, B-3590 Diepenbeek, Belgium. tongxili@sxicc.ac.cn; nianjun.yang@uni-siegen.de |
Keywords: | H2O2 generation;Photocatalysts;Electrocatalysts;Reaction mechanisms | Document URI: | http://hdl.handle.net/1942/40036 | ISSN: | 2311-6706 | e-ISSN: | 2150-5551 | DOI: | 10.1007/s40820-023-01052-2 | ISI #: | 000962535000003 | Rights: | The Author(s) 2023. Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/ licenses/by/4.0/. | Category: | A1 | Type: | Journal Contribution |
| Appears in Collections: | Research publications |
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| Photocatalytic and Electrocatalytic Generation of Hydrogen Peroxide_ Principles, Catalyst Design and Performance.pdf | Published version | 5.17 MB | Adobe PDF | View/Open |
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