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http://hdl.handle.net/1942/41939
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DC Field | Value | Language |
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dc.contributor.author | He, Weikang | - |
dc.contributor.author | Li, Jingjing | - |
dc.contributor.author | Zhang , Yuanyuan | - |
dc.contributor.author | Yang , Juan | - |
dc.contributor.author | Zeng, Ting | - |
dc.contributor.author | YANG, Nianjun | - |
dc.date.accessioned | 2023-12-15T09:15:35Z | - |
dc.date.available | 2023-12-15T09:15:35Z | - |
dc.date.issued | 2023 | - |
dc.date.submitted | 2023-12-15T08:42:49Z | - |
dc.identifier.citation | Small Methods, | - |
dc.identifier.uri | http://hdl.handle.net/1942/41939 | - |
dc.description.abstract | A supercapacitor features high power density and long cycling life. However, its energy density is low. To ensemble a supercapacitor with high power- and energy-densities, the applied capacitor electrodes play the key roles. Herein, a high-performance capacitive electrode is designed and grown on a flexible carbon cloth (CC) substrate via a hydrothermal reaction and a subsequent ion exchange sulfuration process. It has a 3D heterostructure, consisting of sulfur-doped NiMn-layered double hydroxide (LDH) nanosheets (NMLS) and sulfur-doped NiCo-LDH nanowires (NCLS). The electrode with sheet-shaped NMLS and wire-shaped NCLS on their top (NMLS@NCLS/CC) increases the available surface area, providing more pseudocapacitive sites. It exhibits a gravimetric capacity of 555.2 C g-1 at a current density of 1 A g-1, the retention rate of 75.1% when the current density reaches up to 20 A g-1, as well as superior cyclic stability. The assembled asymmetric supercapacitor that is composed of a NMLS@NCLS/CC positive electrode and a sulfurized activated carbon negative electrode presents a maximum energy density of 24.2 Wh kg-1 and a maximum power density of 16000 W kg-1. In this study, a facile strategy for designing hierarchical LDH materials is demonstrated as well as their applications in advanced energy storage systems. On a flexible carbon cloth, sulfur-doped NiMn-layered double hydroxides (LDH) nanosheets (NMLS) and sulfur-doped NiCo-LDH nanosheets (NCLS) are emerged into a 3D heterostructure. Using this NMLS@NCLS/CC positive electrode and a sulfurized activated carbon negative electrode, an ensembled asymmetric supercapacitor features high-performance, including high-power- and energy-densities as well as long-term stability.image | - |
dc.description.sponsorship | This work was financially supported by the Natural Science Foundation of Hubei Province, China (no.2021CFB1192), the Graduate Innovative Fund of Wuhan Institute of Technology of China (CX2022410), Youths Science Foundation of Wuhan Institute of Technology (no.19QD36), and the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation, no. 457444676). | - |
dc.language.iso | en | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.rights | 2023 Wiley-VCH GmbH | - |
dc.subject.other | electrode kinetics | - |
dc.subject.other | energy density | - |
dc.subject.other | supercapacitors | - |
dc.subject.other | transition metal chalcogenides | - |
dc.subject.other | trimetallic layered double hydroxides | - |
dc.title | High-Performance Supercapacitors Using Hierarchical And Sulfur-Doped Trimetallic NiCo/NiMn Layered Double Hydroxides | - |
dc.type | Journal Contribution | - |
local.format.pages | 11 | - |
local.bibliographicCitation.jcat | A1 | - |
dc.description.notes | Zeng, T (corresponding author), Wuhan Inst Technol, Sch Chem & Environm Engn, Hubei Key Lab Novel Reactor & Green Chem Technol, Key Lab Green Chem Proc,Minist Educ, Wuhan 430073, Peoples R China.; Yang, NJ (corresponding author), Hasselt Univ, Dept Chem, B-3590 Diepenbeek, Belgium.; Yang, NJ (corresponding author), Hasselt Univ, IMO IMOMEC, B-3590 Diepenbeek, Belgium. | - |
dc.description.notes | tingzeng1201@wit.edu.cn; nianjun.yang@uhasselt.be | - |
local.publisher.place | POSTFACH 101161, 69451 WEINHEIM, GERMANY | - |
local.type.refereed | Refereed | - |
local.type.specified | Article | - |
local.bibliographicCitation.status | Early view | - |
dc.identifier.doi | 10.1002/smtd.202301167 | - |
dc.identifier.pmid | 38009500 | - |
dc.identifier.isi | 001108653700001 | - |
dc.contributor.orcid | Yang, Nianjun/0000-0002-5558-2314 | - |
local.provider.type | wosris | - |
local.description.affiliation | [He, Weikang; Li, Jingjing; Zhang, Yuanyuan; Yang, Juan; Zeng, Ting] Wuhan Inst Technol, Sch Chem & Environm Engn, Hubei Key Lab Novel Reactor & Green Chem Technol, Key Lab Green Chem Proc,Minist Educ, Wuhan 430073, Peoples R China. | - |
local.description.affiliation | [Yang, Nianjun] Hasselt Univ, Dept Chem, B-3590 Diepenbeek, Belgium. | - |
local.description.affiliation | [Yang, Nianjun] Hasselt Univ, IMO IMOMEC, B-3590 Diepenbeek, Belgium. | - |
local.uhasselt.international | no | - |
item.fullcitation | He, Weikang; Li, Jingjing; Zhang , Yuanyuan; Yang , Juan; Zeng, Ting & YANG, Nianjun (2023) High-Performance Supercapacitors Using Hierarchical And Sulfur-Doped Trimetallic NiCo/NiMn Layered Double Hydroxides. In: Small Methods,. | - |
item.fulltext | With Fulltext | - |
item.contributor | He, Weikang | - |
item.contributor | Li, Jingjing | - |
item.contributor | Zhang , Yuanyuan | - |
item.contributor | Yang , Juan | - |
item.contributor | Zeng, Ting | - |
item.contributor | YANG, Nianjun | - |
item.accessRights | Open Access | - |
crisitem.journal.issn | 2366-9608 | - |
crisitem.journal.eissn | 2366-9608 | - |
Appears in Collections: | Research publications |
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File | Description | Size | Format | |
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Small Methods - 2023 - He - High‐Performance Supercapacitors Using Hierarchical And Sulfur‐Doped Trimetallic NiCo NiMn.pdf Restricted Access | Early view | 10.03 MB | Adobe PDF | View/Open Request a copy |
auteursversie.pdf | Peer-reviewed author version | 20.6 MB | Adobe PDF | View/Open |
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