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http://hdl.handle.net/1942/42919
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DC Field | Value | Language |
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dc.contributor.author | Yang, Shuncheng | - |
dc.contributor.author | Chen, Zhenyu | - |
dc.contributor.author | Zhu, Jintao | - |
dc.contributor.author | Yang, Daobin | - |
dc.contributor.author | Wang, Hongqian | - |
dc.contributor.author | Ding, Pengfei | - |
dc.contributor.author | Wu, Jie | - |
dc.contributor.author | Yan, Pengyu | - |
dc.contributor.author | Xie, Lin | - |
dc.contributor.author | Chen, Fei | - |
dc.contributor.author | WANG, Yuming | - |
dc.contributor.author | Zhang, Jianqi | - |
dc.contributor.author | Ge, Ziyi | - |
dc.date.accessioned | 2024-05-14T07:01:41Z | - |
dc.date.available | 2024-05-14T07:01:41Z | - |
dc.date.issued | 2024 | - |
dc.date.submitted | 2024-05-13T13:09:50Z | - |
dc.identifier.citation | ADVANCED MATERIALS, | - |
dc.identifier.uri | http://hdl.handle.net/1942/42919 | - |
dc.description.abstract | The ternary strategy, in which one guest component is introduced into one host binary system, is considered to be one of the most effective ways to realize high-efficiency organic solar cells (OSCs). To date, there is no efficient method to predict the effectiveness of guest components in ternary OSCs. Herein, three guest compositions (i.e., ANF-1, ANF-2 and ANF-3) with different electrostatic potential (ESP) are designed and synthesized by modulating the electron-withdrawing ability of the terminal groups through density functional theory simulations. The effects of the introduction of guest component into the host system (D18:N3) on the photovoltaic properties are investigated. The theoretical and experimental studies provide a key rule for guest acceptor in ternary OSCs to improve the open-circuit voltage, that is, the larger ESP difference between the guest and host acceptor, the stronger the intermolecular interactions and the higher the miscibility, which improves the luminescent efficiency of the blend film and the electroluminescence quantum yield (EQEEL) of the device by reducing the aggregation-caused-quenching, thereby effectively decreasing the non-radiative voltage loss of ternary OSCs. This work will greatly contribute to the development of highly efficient guest components, thereby promoting the rapid breakthrough of the 20% efficiency bottleneck for single-junction OSCs. A key strategy for predicting efficient guest components to minimize voltage losses in ternary organic solar cells (OSCs) is demonstrated. The larger electrostatic potential (ESP) difference between the guest acceptor and the host acceptor, the smaller non-radiative voltage losses. image | - |
dc.description.sponsorship | S. Yang, Z. Chen and J. Zhu contributed equally to this work. This work was supported by the National Natural Science Foundation of China (No. U21A20331), the National Science Fund for Distinguished Young Scholars (No.21925506), and Zhejiang Provincial Natural Science Foundation of China (No. LQ22E030013), the National Postdoctoral Program for Innovative Talents (No. BX20230386). | - |
dc.language.iso | en | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.rights | 2024 Wiley-VCH Gmb | - |
dc.subject.other | electrostatic potential | - |
dc.subject.other | high miscibility | - |
dc.subject.other | intermolecular interactions | - |
dc.subject.other | non-radiative voltage losses | - |
dc.subject.other | ternary organic solar cells | - |
dc.title | Guest Acceptors with Lower Electrostatic Potential in Ternary Organic Solar Cells for Minimizing Voltage Losses | - |
dc.type | Journal Contribution | - |
local.format.pages | 11 | - |
local.bibliographicCitation.jcat | A1 | - |
dc.description.notes | Yang, DB; Xie, L; Ge, ZY (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Zhejiang Engn Res Ctr Energy Optoelect Mat & Devic, Ningbo 315201, Peoples R China.; Yang, DB; Xie, L; Ge, ZY (corresponding author), Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China.; Wang, YM (corresponding author), Hasselt Univ, Inst Mat Res IMO IMOMEC, Wetenschapspk 1, B-3590 Diepenbeek, Belgium. | - |
dc.description.notes | yangdaobin@nimte.ac.cn; xielin@nimte.ac.cn; yuming.wang@uhasselt.be; | - |
dc.description.notes | geziyi@nimte.ac.cn | - |
local.publisher.place | POSTFACH 101161, 69451 WEINHEIM, GERMANY | - |
local.type.refereed | Refereed | - |
local.type.specified | Article | - |
local.bibliographicCitation.status | Early view | - |
dc.identifier.doi | 10.1002/adma.202401789 | - |
dc.identifier.pmid | 38577904 | - |
dc.identifier.isi | 001200750100001 | - |
dc.contributor.orcid | Yang, Daobin/0000-0001-5611-8209; Wang, Yuming/0000-0001-8096-6144; Zhu, | - |
dc.contributor.orcid | Jintao/0000-0002-3559-1942 | - |
dc.identifier.eissn | 1521-4095 | - |
local.provider.type | wosris | - |
local.description.affiliation | [Yang, Shuncheng] Ningbo Univ, Sch Mat Sci & Chem Engn, Ningbo 315211, Peoples R China. | - |
local.description.affiliation | [Yang, Shuncheng; Chen, Zhenyu; Yang, Daobin; Wang, Hongqian; Ding, Pengfei; Wu, Jie; Yan, Pengyu; Xie, Lin; Ge, Ziyi] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Zhejiang Engn Res Ctr Energy Optoelect Mat & Devic, Ningbo 315201, Peoples R China. | - |
local.description.affiliation | [Chen, Zhenyu; Yang, Daobin; Wang, Hongqian; Ding, Pengfei; Xie, Lin; Ge, Ziyi] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China. | - |
local.description.affiliation | [Zhu, Jintao; Chen, Fei] Univ Nottingham Ningbo China, Dept Chem & Environm Engn, Ningbo 315100, Peoples R China. | - |
local.description.affiliation | [Wang, Yuming] Hasselt Univ, Inst Mat Res IMO IMOMEC, Wetenschapspk 1, B-3590 Diepenbeek, Belgium. | - |
local.description.affiliation | [Zhang, Jianqi] CAS Ctr Excellence Nanosci, Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China. | - |
local.uhasselt.international | yes | - |
item.fulltext | With Fulltext | - |
item.accessRights | Embargoed Access | - |
item.embargoEndDate | 2024-09-05 | - |
item.fullcitation | Yang, Shuncheng; Chen, Zhenyu; Zhu, Jintao; Yang, Daobin; Wang, Hongqian; Ding, Pengfei; Wu, Jie; Yan, Pengyu; Xie, Lin; Chen, Fei; WANG, Yuming; Zhang, Jianqi & Ge, Ziyi (2024) Guest Acceptors with Lower Electrostatic Potential in Ternary Organic Solar Cells for Minimizing Voltage Losses. In: ADVANCED MATERIALS,. | - |
item.contributor | Yang, Shuncheng | - |
item.contributor | Chen, Zhenyu | - |
item.contributor | Zhu, Jintao | - |
item.contributor | Yang, Daobin | - |
item.contributor | Wang, Hongqian | - |
item.contributor | Ding, Pengfei | - |
item.contributor | Wu, Jie | - |
item.contributor | Yan, Pengyu | - |
item.contributor | Xie, Lin | - |
item.contributor | Chen, Fei | - |
item.contributor | WANG, Yuming | - |
item.contributor | Zhang, Jianqi | - |
item.contributor | Ge, Ziyi | - |
crisitem.journal.issn | 0935-9648 | - |
crisitem.journal.eissn | 1521-4095 | - |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
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Advanced Materials - 2024 - Yang - Guest Acceptors with Lower Electrostatic Potential in Ternary Organic Solar Cells for.pdf Restricted Access | Published version | 4.33 MB | Adobe PDF | View/Open Request a copy |
auteursversie.pdf Until 2024-09-05 | Peer-reviewed author version | 1.81 MB | Adobe PDF | View/Open Request a copy |
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