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http://hdl.handle.net/1942/42926
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DC Field | Value | Language |
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dc.contributor.author | Ge, Bingcheng | - |
dc.contributor.author | Hu, Liang | - |
dc.contributor.author | Yu, Xiaoliang | - |
dc.contributor.author | Wang, Lixu | - |
dc.contributor.author | Fernandez, Carlos | - |
dc.contributor.author | YANG, Nianjun | - |
dc.contributor.author | Liang, Qinghua | - |
dc.contributor.author | Yang, Quan‐Hong | - |
dc.date.accessioned | 2024-05-14T10:30:23Z | - |
dc.date.available | 2024-05-14T10:30:23Z | - |
dc.date.issued | 2024 | - |
dc.date.submitted | 2024-04-23T09:05:22Z | - |
dc.identifier.citation | ADVANCED MATERIALS, | - |
dc.identifier.issn | 0935-9648 | - |
dc.identifier.uri | http://hdl.handle.net/1942/42926 | - |
dc.description.abstract | Alkali metal–air batteries (AMABs) promise ultrahigh gravimetric energydensities, while the inherent poor cycle stability hinders their practicalapplication. To address this challenge, most previous efforts are devoted toadvancing the air cathodes with high electrocatalytic activity. Recent studieshave underlined the solid–liquid–gas triple-phase interface around the anodecan play far more significant roles than previously acknowledged by thescientific community. Besides the bottlenecks of uncontrollable dendritegrowth and gas evolution in conventional alkali metal batteries, the corrosivegases, intermediate oxygen species, and redox mediators in AMABs causemore severe anode corrosion and structural collapse, posing greaterchallenges to the stabilization of the anode triple-phase interface. This workaims to provide a timely perspective on the anode interface engineering fordurable AMABs. Taking the Li–air battery as a typical example, this criticalreview shows the latest developed anode stabilization strategies, includingformulating electrolytes to build protective interphases, fabricating advancedanodes to improve their anti-corrosion capability, and designing functionalseparator to shield the corrosive species. Finally, the remaining scientific andtechnical issues from the prospects of anode interface engineering arehighlighted, particularly materials system engineering, for the practical use ofAMABs | - |
dc.description.sponsorship | The authors gratefully acknowledge financial support from The HongKong Polytechnic University (ZZLM, YY5K), Local Science and TechnologyDevelopment Project of the Central Government (No. 2022ZY0011),Natural Science Foundation of Guangdong (No. 2023A1515010020),Innovation and Technology Fund (ITS-325-22FP). Q.L. thanks the finan-cial support from the Natural Science Foundation of Jiangxi Province(No. 20232ACB214001), the Research fund from Jingxi Province HumanResources and Social Security Department, and the Chinese Academy ofSciences. Q.-H.Y. is grateful to the National Natural Science Foundationof China (No. 51932005) | - |
dc.language.iso | en | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.rights | 2024 Wiley-VCH GmbH2400937 | - |
dc.subject.other | alkali metal–air batteries | - |
dc.subject.other | anode engineering | - |
dc.subject.other | electrolyte formulation | - |
dc.subject.other | func-tional separator | - |
dc.subject.other | triple-phase interfaces | - |
dc.title | Engineering Triple‐Phase Interfaces around the Anode towards Practical Alkali Metal‐Air Batteries | - |
dc.type | Journal Contribution | - |
local.bibliographicCitation.jcat | A1 | - |
dc.description.notes | Yu, XL (corresponding author), Hong Kong Polytech Univ, Dept Mech Engn, Hong Kong 999077, Peoples R China.; Yu, XL (corresponding author), Hong Kong Polytech Univ, Res Inst Smart Energy, Hong Kong 999077, Peoples R China.; Liang, QH (corresponding author), Chinese Acad Sci, Ganjiang Innovat Acad, Key Lab Rare Earth, Ganzhou 341000, Jiangxi, Peoples R China.; Yang, QH (corresponding author), Tianjin Univ, Sch Chem Engn & Technol, Tianjin Key Lab Adv Carbon & Electrochem Energy St, Nanoyang Grp, Tianjin 300072, Peoples R China. | - |
dc.description.notes | xiaoliang.yu@polyu.edu.hk; qhliang@gia.cas.cn; qhyangcn@tju.edu.cn | - |
local.publisher.place | POSTFACH 101161, 69451 WEINHEIM, GERMANY | - |
local.type.refereed | Refereed | - |
local.type.specified | Review | - |
local.bibliographicCitation.status | Early view | - |
dc.identifier.doi | 10.1002/adma.202400937 | - |
dc.identifier.isi | 001209443700001 | - |
dc.identifier.eissn | 1521-4095 | - |
local.provider.type | CrossRef | - |
local.description.affiliation | [Ge, Bingcheng; Hu, Liang; Yu, Xiaoliang] Hong Kong Polytech Univ, Dept Mech Engn, Hong Kong 999077, Peoples R China. | - |
local.description.affiliation | [Ge, Bingcheng; Hu, Liang; Yu, Xiaoliang] Hong Kong Polytech Univ, Res Inst Smart Energy, Hong Kong 999077, Peoples R China. | - |
local.description.affiliation | [Wang, Lixu] Fujian XFH New Energy Mat Co Ltd, 38 Shuidong Ind Pk, Yongan 366000, Peoples R China. | - |
local.description.affiliation | [Fernandez, Carlos] Robert Gordon Univ, Sch Pharm Life Sci, Aberdeen AB10 7QB, Scotland. | - |
local.description.affiliation | [Yang, Nianjun] Hasselt Univ, Dept Chem, B-3590 Diepenbeek, Belgium. | - |
local.description.affiliation | [Liang, Qinghua] Chinese Acad Sci, Ganjiang Innovat Acad, Key Lab Rare Earth, Ganzhou 341000, Jiangxi, Peoples R China. | - |
local.description.affiliation | [Yang, Quan-Hong] Tianjin Univ, Sch Chem Engn & Technol, Tianjin Key Lab Adv Carbon & Electrochem Energy St, Nanoyang Grp, Tianjin 300072, Peoples R China. | - |
local.uhasselt.international | yes | - |
item.fullcitation | Ge, Bingcheng; Hu, Liang; Yu, Xiaoliang; Wang, Lixu; Fernandez, Carlos; YANG, Nianjun; Liang, Qinghua & Yang, Quan‐Hong (2024) Engineering Triple‐Phase Interfaces around the Anode towards Practical Alkali Metal‐Air Batteries. In: ADVANCED MATERIALS,. | - |
item.accessRights | Embargoed Access | - |
item.contributor | Ge, Bingcheng | - |
item.contributor | Hu, Liang | - |
item.contributor | Yu, Xiaoliang | - |
item.contributor | Wang, Lixu | - |
item.contributor | Fernandez, Carlos | - |
item.contributor | YANG, Nianjun | - |
item.contributor | Liang, Qinghua | - |
item.contributor | Yang, Quan‐Hong | - |
item.embargoEndDate | 2024-11-14 | - |
item.fulltext | With Fulltext | - |
crisitem.journal.issn | 0935-9648 | - |
crisitem.journal.eissn | 1521-4095 | - |
Appears in Collections: | Research publications |
Files in This Item:
File | Description | Size | Format | |
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Revised Manuscript-Final version.docx Until 2024-11-14 | Peer-reviewed author version | 11.54 MB | Microsoft Word | View/Open Request a copy |
Advanced Materials - 2024 - Ge - Engineering Triple‐Phase Interfaces around the Anode toward Practical Alkali Metal Air (1).pdf Restricted Access | Published version | 10.36 MB | Adobe PDF | View/Open Request a copy |
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