Please use this identifier to cite or link to this item: http://hdl.handle.net/1942/42985
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dc.contributor.authorLian, Xinxin-
dc.contributor.authorXu, Ye-
dc.contributor.authorFu, Wei-
dc.contributor.authorMeng, Rui-
dc.contributor.authorMa, Quanxing-
dc.contributor.authorXu , Chunyu-
dc.contributor.authorLuo, Ming-
dc.contributor.authorHu, Ying-
dc.contributor.authorHan, Junchao-
dc.contributor.authorMin, Hao-
dc.contributor.authorKRISHNA, Anurag-
dc.contributor.authorChen, Yifan-
dc.contributor.authorZhou, Huawei-
dc.contributor.authorZhang , Xueling-
dc.contributor.authorChen , Cong-
dc.contributor.authorChang, Jin-
dc.contributor.authorLi, Can-
dc.contributor.authorChen, Yifeng-
dc.contributor.authorFeng, Zhiqiang-
dc.contributor.authorLi, Zhen-
dc.contributor.authorZuo, Guangzheng-
dc.contributor.authorGao, Jifan-
dc.contributor.authorMo, Xiaoliang-
dc.contributor.authorZhang , Hong-
dc.contributor.authorChu, Junhao-
dc.date.accessioned2024-05-22T11:01:19Z-
dc.date.available2024-05-22T11:01:19Z-
dc.date.issued2024-
dc.date.submitted2024-05-15T09:15:03Z-
dc.identifier.citationADVANCED FUNCTIONAL MATERIALS,-
dc.identifier.issn1616-301X-
dc.identifier.urihttp://hdl.handle.net/1942/42985-
dc.description.abstractA facile and eco-friendly dimethyl sulfoxide-mediated solution aging (DMSA) treatment is presented to control the crystallization dynamics of methylammonium (MA)-free wide-bandgap (WBG) perovskite films, enhancing film quality, and morphology for high-performance tandem solar cells. The comprehensive structural, morphological, and characterization analyses reveal that the DMSA treatment significantly enhances composition and morphology homogeneity while suppressing halide segregation. Consequently, opaque, and semi-transparent MA-free WBG perovskite solar cells (PSCs) exhibit remarkable power conversion efficiencies (PCEs) of 18.28% and 17.61%, respectively. Notably, the unencapsulated DMSA-treated devices maintain 95% of the initial PCE after 900 h of continuous operation at 55 degrees C +/- 5 degrees C. Furthermore, stacking semi-transparent DMSA-treated PSCs as top cells in a 4T tandem configuration, along with silicon heterojunction (SHJ), lead-tin (Pb-Sn) alloyed PSCs, and organic photovoltaics (OPV) as bottom cells, yields impressive PCEs of 28.09%, 26.09%, and 25.28%, respectively, for the fabricated tandem cells. This innovative approach opens new avenues for enhancing the photo-stability and photovoltaic performance of perovskite-based tandem solar cells. A facile and eco-friendly dimethyl sulfoxide-mediated solution aging (DMSA) treatment is proposed to homogenize the morphology and composition of methylammonium-free wide-bandgap perovskite films, which contributes to highly efficient and stable semitransparent perovskite solar cells and tandem solar cells. image-
dc.description.sponsorshipAcknowledgements This work was supported by Shanghai Pujiang Program (22PJ1401200) and the National Natural Science Foundation of China (No. 52302229).-
dc.language.isoen-
dc.publisherWILEY-V C H VERLAG GMBH-
dc.rights2024 Wiley-VCH GmbH-
dc.subject.otherhomogeneity-
dc.subject.othermethylammonium-free-
dc.subject.otherperovskite solar cells-
dc.subject.othertandem solar cellswide-bandgap perovskite-
dc.titleHomogenizing Morphology and Composition of Methylammonium-Free Wide-Bandgap Perovskite for Efficient and Stable Tandem Solar Cells-
dc.typeJournal Contribution-
local.format.pages11-
local.bibliographicCitation.jcatA1-
dc.description.notesZhang, H; Mo, XL (corresponding author), Fudan Univ, State Key Lab Photovolta Sci & Technol, Shanghai Frontiers Sci Res Base Intelligent Optoel, Dept Mat Sci,Inst Optoelect,Yiwu Res Inst, Shanghai 200433, Peoples R China.-
dc.description.noteshzhangioe@fudan.edu.cn; xlmo@fudan.edu.cn-
local.publisher.placePOSTFACH 101161, 69451 WEINHEIM, GERMANY-
local.type.refereedRefereed-
local.type.specifiedArticle-
local.bibliographicCitation.statusEarly view-
dc.identifier.doi10.1002/adfm.202402061-
dc.identifier.isi001204838900001-
dc.contributor.orcidKrishna, Anurag/0000-0001-7255-7412-
dc.identifier.eissn1616-3028-
dc.identifier.eissn1616-3028-
local.provider.typewosris-
local.description.affiliation[Lian, Xinxin; Ma, Quanxing; Xu, Chunyu; Luo, Ming; Hu, Ying; Han, Junchao; Chen, Yifan; Zhang, Hong; Mo, Xiaoliang; Chu, Junhao] Fudan Univ, State Key Lab Photovolta Sci & Technol, Shanghai Frontiers Sci Res Base Intelligent Optoel, Dept Mat Sci,Inst Optoelect,Yiwu Res Inst, Shanghai 200433, Peoples R China.-
local.description.affiliation[Xu, Ye; Zhang, Xueling; Chen, Yifeng; Feng, Zhiqiang; Gao, Jifan] Trina Solar, State Key Lab Photovolta Sci & Technol, Changzhou 213031, Peoples R China.-
local.description.affiliation[Fu, Wei; Zuo, Guangzheng] Fudan Univ, Inst Elect Light Sources, Sch Informat Sci & Technol, Shanghai 200433, Peoples R China.-
local.description.affiliation[Meng, Rui; Li, Can; Li, Zhen] Northwestern Polytech Univ, Ctr Nano Energy Mat, Sch Mat Sci & Engn, State Key Lab Solidificat Proc, Xian 710072, Peoples R China.-
local.description.affiliation[Meng, Rui; Li, Can; Li, Zhen] Shaanxi Joint Lab Graphene NPU, Xian 710072, Peoples R China.-
local.description.affiliation[Ma, Quanxing; Chen, Cong] Hebei Univ Technol, Sch Mat Sci & Engn, State Key Lab Reliabil & Intelligence Elect Equipm, Tianjin 300130, Peoples R China.-
local.description.affiliation[Min, Hao; Chang, Jin] Nanjing Tech Univ, Inst Adv Mat IAM, Key Lab Flexible Elect KLOFE, Nanjing 211816, Peoples R China.-
local.description.affiliation[Min, Hao; Chang, Jin] Nanjing Tech Univ, Sch Flexible Elect Future Technol, Nanjing 211816, Peoples R China.-
local.description.affiliation[Krishna, Anurag] Imo Imomec, Imec, Thin Film PV Technol, Thor Pk 8320, B-3600 Genk, Belgium.-
local.description.affiliation[Krishna, Anurag] Imo Imomec, EnergyVille, Thor Pk 8320, B-3600 Genk, Belgium.-
local.description.affiliation[Krishna, Anurag] Hasselt Univ, Imo Imomec, Martelarenlaan 42, B-3500 Hasselt, Belgium.-
local.description.affiliation[Zhou, Huawei] Liaocheng Univ, Coll Mat Sci & Engn, Sch Chem & Chem Engn, Shandong Prov Key Lab,Collaborat Innovat Ctr Chem, Liaocheng 252000, Peoples R China.-
local.uhasselt.internationalyes-
item.accessRightsEmbargoed Access-
item.contributorLian, Xinxin-
item.contributorXu, Ye-
item.contributorFu, Wei-
item.contributorMeng, Rui-
item.contributorMa, Quanxing-
item.contributorXu , Chunyu-
item.contributorLuo, Ming-
item.contributorHu, Ying-
item.contributorHan, Junchao-
item.contributorMin, Hao-
item.contributorKRISHNA, Anurag-
item.contributorChen, Yifan-
item.contributorZhou, Huawei-
item.contributorZhang , Xueling-
item.contributorChen , Cong-
item.contributorChang, Jin-
item.contributorLi, Can-
item.contributorChen, Yifeng-
item.contributorFeng, Zhiqiang-
item.contributorLi, Zhen-
item.contributorZuo, Guangzheng-
item.contributorGao, Jifan-
item.contributorMo, Xiaoliang-
item.contributorZhang , Hong-
item.contributorChu, Junhao-
item.embargoEndDate2024-10-18-
item.fulltextWith Fulltext-
item.fullcitationLian, Xinxin; Xu, Ye; Fu, Wei; Meng, Rui; Ma, Quanxing; Xu , Chunyu; Luo, Ming; Hu, Ying; Han, Junchao; Min, Hao; KRISHNA, Anurag; Chen, Yifan; Zhou, Huawei; Zhang , Xueling; Chen , Cong; Chang, Jin; Li, Can; Chen, Yifeng; Feng, Zhiqiang; Li, Zhen; Zuo, Guangzheng; Gao, Jifan; Mo, Xiaoliang; Zhang , Hong & Chu, Junhao (2024) Homogenizing Morphology and Composition of Methylammonium-Free Wide-Bandgap Perovskite for Efficient and Stable Tandem Solar Cells. In: ADVANCED FUNCTIONAL MATERIALS,.-
crisitem.journal.issn1616-301X-
crisitem.journal.eissn1616-3028-
Appears in Collections:Research publications
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AFM accepted version_WBG.pdf
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