Please use this identifier to cite or link to this item: http://hdl.handle.net/1942/15828
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dc.contributor.authorBECKER, Thijs-
dc.contributor.authorNELISSEN, Kwinten-
dc.contributor.authorCLEUREN, Bart-
dc.contributor.authorPARTOENS, Bart-
dc.contributor.authorVAN DEN BROECK, Christian-
dc.date.accessioned2013-10-17T14:07:14Z-
dc.date.available2013-10-17T14:07:14Z-
dc.date.issued2013-
dc.identifier.citationPHYSICAL REVIEW LETTERS, 111 (11)-
dc.identifier.issn0031-9007-
dc.identifier.urihttp://hdl.handle.net/1942/15828-
dc.description.abstractWe evaluate the self-diffusion and transport diffusion of interacting particles in a discrete geometry consisting of a linear chain of cavities, with interactions within a cavity described by a free-energy function. Exact analytical expressions are obtained in the absence of correlations, showing that the self- diffusion can exceed the transport diffusion if the free-energy function is concave. The effect of correlations is elucidated by comparison with numerical results. Quantitative agreement is obtained with recent experimental data for diffusion in a nanoporous zeolitic imidazolate framework material, ZIF-8.-
dc.description.sponsorshipThis work was supported by the Flemish Science Foundation (FWO-Vlaanderen).-
dc.language.isoen-
dc.titleDiffusion of Interacting Particles in Discrete Geometries-
dc.typeJournal Contribution-
dc.identifier.issue11-
dc.identifier.spageArt. N° 110601-
dc.identifier.volume111-
local.format.pages5-
local.bibliographicCitation.jcatA1-
dc.description.notes[Becker, T.; Nelissen, K.; Cleuren, B.; Van den Broeck, C.] Hasselt Univ, B-3590 Diepenbeek, Belgium. [Nelissen, K.; Partoens, B.] Univ. Antwerpen, B-2020 Antwerpen, Belgium-
local.type.refereedRefereed-
local.type.specifiedArticle-
dc.identifier.doi10.1103/PhysRevLett.111.110601-
dc.identifier.isi000324233800001-
item.fulltextWith Fulltext-
item.contributorBECKER, Thijs-
item.contributorNELISSEN, Kwinten-
item.contributorCLEUREN, Bart-
item.contributorPARTOENS, Bart-
item.contributorVAN DEN BROECK, Christian-
item.validationecoom 2014-
item.accessRightsOpen Access-
item.fullcitationBECKER, Thijs; NELISSEN, Kwinten; CLEUREN, Bart; PARTOENS, Bart & VAN DEN BROECK, Christian (2013) Diffusion of Interacting Particles in Discrete Geometries. In: PHYSICAL REVIEW LETTERS, 111 (11).-
crisitem.journal.issn0031-9007-
crisitem.journal.eissn1079-7114-
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