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http://hdl.handle.net/1942/36864
Title: | One-pot multifunctional polyesters by continuous flow organocatalysed ring-opening polymerisation for targeted and tunable materials design | Authors: | Bakkali-Hassani, Camille Hooker, Jordan P. Voorter, Pieter-Jan RUBENS, Maarten Cameron, Neil R. JUNKERS, Tanja |
Issue Date: | 2022 | Publisher: | ROYAL SOC CHEMISTRY | Source: | Polymer chemistry, 13 (10) , p. 1387-1393 | Abstract: | Targeted and tunable access to biodegradable polymers will be vital for their continued adoption and use in modern materials applications. Herein we report a platform for the synthesis of well-defined, curable biodegradable polymer precursors, prepared in a controlled manner via continuous flow ring-opening polymerisation/post-modification reactions of epsilon-caprolactone and L-lactide. Polymer architectures are characterised by H-1 NMR spectroscopy, ESI mass spectrometry, and size exclusion chromatography, and their potential application in materials synthesis is subsequently highlighted by employing them as precursors to prepare networks and polymerised high internal phase emulsions (polyHIPEs) via an emulsion templating strategy using photo-initiated thiol-ene click reaction. | Notes: | Bakkali-Hassani, C; Junkers, T (corresponding author), Monash Univ, Sch Chem, Polymer React Design Grp, 19 Rainforest Walk, Clayton, Vic 3800, Australia.; Bakkali-Hassani, C; Cameron, NR (corresponding author), Monash Univ, Dept Mat Sci & Engn, Clayton, Vic 3800, Australia.; Junkers, T (corresponding author), Hasselt Univ, Materlarenlaan 42, B-3500 Hasselt, Belgium.; Cameron, NR (corresponding author), Univ Warwick, Sch Engn, Coventry CV4 7AL, W Midlands, England. tanja.junkers@monash.edu |
Document URI: | http://hdl.handle.net/1942/36864 | ISSN: | 1759-9954 | e-ISSN: | 1759-9962 | DOI: | 10.1039/d2py00088a | ISI #: | WOS:000755737400001 | Rights: | The Royal Society of Chemistry 2022 | Category: | A1 | Type: | Journal Contribution | Validations: | ecoom 2023 |
Appears in Collections: | Research publications |
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d2py00088a 1387..1393 ++.pdf Restricted Access | Published version | 2.52 MB | Adobe PDF | View/Open Request a copy |
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